Harry Dankowicz [email] (Dept. of Mechanical and Industrial Engineering, UIUC) Near-Grazing Dynamics in Tapping-Mode Atomic Force Microscopy Abstract: > Nanostructured materials and devices can be endowed with novel physical properties that make them suitable for a wide range of applications. Carbon nanostructures exhibit hydrogen-adsorbing characteristics that make them attractive candidates as storage devices in a hydrogen-fuel supply chain. Similarly, self-assembly of ferromagnetic nanoparticles is a promising technique for producing high-density magnetic data storage devices and biomedical materials with desirable surface properties. > > Characterization techniques of carbon nanotubes through electron microscopy are tedious and destroy the sample integrity. Similarly, as many of the structures resulting from self assembly of nanoparticles are soft and fragile, their topography can be damaged by the use of conventional nanoscale materials characterization instrumentation. > > Less destructive characterization is possible using scanning-probe microscopy, e.g., intermittent-contact (TappingModeTM) atomic-force microscopy. Here, however, nonlinear effects due to large variations in the force field on the probe tip over very small length scales and the intermittency of contact may induce strong dynamical instabilities. These can result in a sudden loss of stability of low-contact-velocity oscillations of the atomic-force-microscope tip in favor of oscillations with high contact velocity and destructive, nonrepeatable, and unreliable characterization of the nanostructure. > > In tapping-mode microscopy, the onset of instability can be traced to a critical choice of values for system parameters, for which a periodic trajectory exists that achieves zero-normal-velocity (grazing) contact with a system discontinuity. Dynamical-systems methods for the analysis of mechanical and physical systems with intermittent contact can be employed to formulate normal-form descriptions of the near-grazing dynamics that capture the destabilizing effects of contact (cf. [1, 2], but see also [3]). In particular, near-grazing dynamics can be analyzed through the introduction of a discontinuity mapping that i) captures the local dynamics in the vicinity of the grazing contact including variations in time-of-flight to the discontinuity and the contact behavior; ii) can be entirely characterized by conditions at the grazing contact; iii) is nonsmooth in the deviation from the point of grazing contact; and iv) can be studied to arbitrary order of accuracy. > > In this talk, a discontinuity-mapping analysis is employed to investigate the near-grazing dynamics in a lumped-mass model of an oscillating atomic-force-microscope cantilever tip interacting with a sample surface. Here, surface interactions are modeled through a combination of the attraction due to van-der-Waals forces and the repulsion due to Pauli and ionic exclusion. Two different normal forms are derived that capture the critical transition between non-contact oscillations that experience only surface attraction and intermittent-contact oscillations that also experience the repelling response of the sample. The analysis predicts the loss of stability associated with near-grazing contact and suggests ways to suppress such loss through passive redesign and active control. > 1. Dankowicz, H. and Nordmark, A.B., "On the origin and bifurcations of stick-slip oscillations," Physica D 136(3-4), pp. 280-302, 2000. > 2. di Bernardo, M., Budd, C.J., and Champneys, A.R., "Normal form maps for grazing bifurcations in n-dimensional piecewise-smooth dynamical systems," Physica D 160(3-4), pp. 222-254, 2001. > 3. van de Water, W. and Molenaar, J., "Dynamics of vibrating atomic force microscopy," Nanotechnology, 11, pp. 192-199, 2000. |
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